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Beilstein J. Org. Chem. 2016, 12, 2372–2377, doi:10.3762/bjoc.12.231
Graphical Abstract
Scheme 1: Synthesis of N-phosphonyl-β-amino Weinreb amides.
Scheme 2: Aminochlorination of α,β-unsaturated ketones in ionic liquid.
Scheme 3: Conversion of β-amino Weinreb amides to aziridines.
Figure 1: Possible hydrogen bonding conformation.
Scheme 4: Resonance structures of Weinreb amides.
Scheme 5: Transformation of trans-aziridine.
Scheme 6: Proposed mechanism of aminochlorination of α,β-unsaturated Weinreb amides.